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Local Plastic Response and Slow Heterogeneous Dynamics of Supercooled Liquids

Articolo
Data di Pubblicazione:
2022
Abstract:
We demonstrate, via numerical simulations, that the relaxation dynamics of supercooled liquids correlates well with a plastic length scale measuring a particle's response to impulsive localized perturbations and weakly to measures of local elasticity. We find that the particle averaged plastic length scale vanishes linearly in temperature and controls the super-Arrhenius temperature dependence of the relaxation time. Furthermore, we show that the plastic length scale of individual particles correlates with their typical displacement at the relaxation time. In contrast, the local elastic response only correlates with the dynamics on the vibrational timescale.
Tipologia CRIS:
01.01 Articolo in rivista
Keywords:
-
Elenco autori:
PICA CIAMARRA, Massimo
Autori di Ateneo:
PICA CIAMARRA MASSIMO
Link alla scheda completa:
https://iris.cnr.it/handle/20.500.14243/416766
Pubblicato in:
PHYSICAL REVIEW LETTERS (PRINT)
Journal
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http://www.scopus.com/inward/record.url?eid=2-s2.0-85133500369&partnerID=q2rCbXpz
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